Correlated multielectron systems in strong laser fields: A multiconfiguration time-dependent Hartree-Fock approach
摘要:
The multiconfiguration time-dependent Hartree-Fock approach for the description of correlated few-electron dynamics in the presence of strong laser fields is introduced and a comprehensive description of the method is given. Total ionization and electron spectra for the ground and first excited ionic channels are calculated for one-dimensional model systems with up to six active electrons. Strong correlation effects are found in the shape of photoelectron peaks and the dependence of ionization on molecule size.
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关键词:
atomic and molecular physics correlations electron spectra electrons hartree-fock method ionization laser radiation molecules one-dimensional calculations time dependence
DOI:
10.1103/PhysRevA.71.012712
被引量:
年份:
2005
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