Phase-Sensitive Observation of a Spin-Orbital Mott State in Sr2IrO4

阅读量:

90

作者:

BJ KimH OhsumiT KomesuS SakaiT MoritaH TakagiT Arima

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摘要:

Measurement of the quantum-mechanical phase in quantum matter provides the most direct manifestation of the underlying abstract physics. We used resonant x-ray scattering to probe the relative phases of constituent atomic orbitals in an electronic wave function, which uncovers the unconventional Mott insulating state induced by relativistic spin-orbit coupling in the layered 5d transition metal oxide SrIrO. A selection rule based on intra-atomic interference effects establishes a complex spin-orbital state represented by an effective total angular momentum = 1/2 quantum number, the phase of which can lead to a quantum topological state of matter.

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DOI:

10.1126/science.1167106

被引量:

462

年份:

2009

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2013
被引量:85

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