Experimental and Theoretical Investigations of the Sulfite-Based Polyoxometalate Cluster Redox Series: α- and β-[Mo18O54(SO3)2]4−/5−/6−
阅读量：
26
摘要：
The synthesis, isolation and structural characterization of the sulfite polyoxomolybdate clusters -(D3h)(C20H44N)4{-[Mo18O54(SO3)2]}CH3CN and β-(D3d)(C20H44N)4{β-[Mo18O54(SO3)2]}CH3CN is presented. Voltammetric studies in acetonitrile (0.1 M Hx4NClO4, Hx4N=tetra-n-hexylammonium) reveal the presence of an extensive series of six one-elec
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关键词：
density functional calculations electrochemistry EPR spectroscopy molybdenum polyoxometalates sulfite
DOI：
10.1002/chem.200501450
被引量：
年份：
2006
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